Long-term (2008-2018) aerosol properties and radiative effect at high-altitude sites over western trans-Himalayas
["Dumka, U. C","Ningombam, Shantikumar S","Kaskaoutis, D. G","Madhavan, B. L","Song, H-J","Angchuk, Dorje","Jorphail, Sonam"]
2020-09-10
期刊论文
Analysis of the climatology of aerosol properties is performed over Hanle (4500 m) and Merak (4310 m), two remote-background sites in the western trans-Himalayas, based on eleven years (2008-2018) of sun/sky radiometer (POM-01, Prede) measurements. The two sites present very similar atmospheric conditions and aerosol properties allowing us to examine them as continuous single-data series. The annual average aerosol optical depth at 500 nm (AOD(500)) is 0.04 +/- 0.03, associated with an Angstrom exponent (AE(440-870)) of 0.58 +/- 0.35 and a single scattering albedo (SSA(500)) of 0.95 +/- 0.05. AOD(500) exhibits higher values in May (similar to 0.07) and lower in winter (similar to 0.03), while AE(400-870) minimizes in spring, indicating influence by coarse-mode dust aerosols, either emitted regionally or long-range transported. The de-convolution of AOD(500) into fine and coarse modes justifies the aerosol seasonality and sources, while the marginal diurnal variation in all aerosol properties reveals a weak influence from local sources, except for some few aerosol episodes. The aerosol-volume size distribution presents a mode value at similar to 10 mu m with secondary peaks at accumulation (similar to 2 mu m) and fine modes (similar to 0.03 mu m) and low variability between the seasons. A classification of the aerosol types based on the fine-mode fraction (FMF) vs. SSA(500) relationship reveals the dominance of aerosols in the FMF range of 0.4-0.6, characterized as mixed (39%), followed by fine aerosols with high scattering efficiency (26%), while particles related to dust contribute similar to 21%, with low fractions of fine-absorbing aerosols (similar to 13%). The aerosol radiative forcing (ARF) estimates reveal a small cooling effect at the top of the atmosphere (-1.3 Wm(-2)), while at the surface, the ARF ranges from -2 Wm(-2) to -6 Wm(-2) on monthly basis. The monthly-mean atmospheric radiative forcing (similar to 1 to 4 Wm(-2)) leads to heating rates of 0.04 to 0.13 K day(-1). These ARF values are higher than the global averages and may cause climate implications over the trans-Himalayan region. (C) 2020 Elsevier B.V. All rights reserved.
来源平台:SCIENCE OF THE TOTAL ENVIRONMENT