新型两亲嵌段共聚物纳米纤维膜材对环境雌激素的吸附及机理研究

难降解污染物 环境雌激素 两亲嵌段共聚物 纳米纤维膜 吸附
孙姣霞 2016-01 项目
Estrogens, as one typical endocrine disrupting compounds, having the persistence and refractory characteristics, could lead to the endocrine disorders and feminization of animal even at ng/L levels, so it brings about a big threat to water quality assurance and ecological security. One of the contemporary focal issue and difficults is researching more efficent absorbents for removal the estrogens and understand the absorption mechanism. In our study, considering the interaction of estrogens and the polymer absorbents, we design a novel amphiphilic block copolymer. Meanwhile, the novel amphiphilic block copolymer is modifed by β-cyclodextrin-NH2 (β-CD) by green grafting reaction in mild condition for facilitated the absorption of estrogens. The hydrophility and hydrophobicity of the copolymer is adjusted by changing the ratio of hydrophilic block and hydrophobic block. The content of β-CD is controlled by the reaction condition. Combining the modern nanotechnology, the nano and micro fibers membrance from copolymers are prepared by electrospinning. Three typical estrogens are used as research subjects. The relationship of copolymer molecular formula and estrogens are illustrated and further infer the sorption mechnism, which will lay a foundation for the polymer as absorbents for deeply removal the estrogens for water.
环境雌激素是在水循环过程中长期存在、难降解的一类典型内分泌干扰素,它即使在极低的浓度下可能导致动物内分泌紊乱及雌性化的趋势,因而对水体和生态安全构成很大威胁。开发高效的吸附材料去除环境水体中的雌激素并明确其吸附机理是目前研究的热点和难点之一。本课题针对典型雌激素的分子特征,基于聚合物与典型环境雌激素可能发生的相互作用,从分子角度设计一种新型两亲嵌段共聚物,并通过绿色接枝具有包络能力的环糊精,促进其对环境雌激素的吸附。通过改变亲疏水嵌段比例,调节材料的亲疏水性;通过控制反应条件,调节环糊精的接枝量。结合现代纳米电纺技术,将合成的聚合物材料通过静电纺丝,制备微纳孔结合的纳米纤维薄膜。以三种典型环境雌激素为研究对象,通过精确控制材料的分子组成和物理结构,从理化性质两方面共同阐明材料与环境雌激素的关系,进而推断吸附机理,为材料在深化处理水体中环境雌激素的应用奠定基础。