The study of urban aerosol and its influence on radiation and meteorological regime is important due to the climate effect. Using COSMO-ART model with TERRA_URB parameterization, we estimated aerosols and their radiative and temperature response at different emission levels in Moscow. Mean urban aerosol optical depth (AOD) was about 0.029 comprising 20-30% of the total AOD. Urban black carbon mass concentration and urban PM10 accounted for 86% and 74% of their total amount, respectively. The urban AOD provided negative shortwave effective radiative forcing (ERF) of -0.9 W m(-2) at the top of the atmosphere (TOA) for weakly absorbing aerosol and positive ERF for highly absorbing aerosol. Urban canopy effects decreased surface albedo from 19.1% to 16.9%, which resulted in positive shortwave ERF at TOA, while for longwave irradiance negative ERF was observed due to additional emitting of urban heat. Air temperature at 2 m decreased independently on the ERF sign, partially compensating (up to 0.5 degrees C) for urban heat island effect (1.5 degrees C) during daytime. Mean radiative atmospheric absorption over the Moscow center in clear sky conditions reaches 4 W m(-2) due to urban AOD. The study highlights the role of urban aerosol and its radiative and temperature effects.

Since China implemented the Air Pollution Prevention and Control Action Plan in 2013, the aerosol emis-sions in East Asia have been greatly reduced, while emissions in South Asia have continued to increase. This has led to a dipole pattern of aerosol emissions between South Asia and East Asia. Here, the East Asian summer monsoon (EASM) responses to the dipole changes in aerosol emissions during 2013-17 are investigated using the atmosphere model of Com-munity Earth System Model version 2 (CESM2). We show that decreases in East Asian emissions alone lead to a positive aerosol effective radiative forcing (ERF) of 1.59 (+/- 0.97) W m-2 over central-eastern China (25 degrees-40 degrees N, 105 degrees-122.5 degrees E), along with a 0.09 (+/- 0.07)degrees C warming in summer during 2013-17. The warming intensified the land-sea thermal contrast and increased the rainfall by 0.32 (+/- 0.16) mm day-1. When considering both the emission reductions in East Asia and in-creases in South Asia, the ERF is increased to 3.39 (+/- 0.89) W m-2, along with an enhanced warming of 0.20 (+/- 0.08)degrees C over central-eastern China, while the rainfall insignificant decreased by 0.07 (+/- 0.16) mm day-1. It is due to the westward shift of the strengthened western Pacific subtropical high, linked to the increase in black carbon in South Asia. Based on multiple EASM indices, the reductions in aerosol emissions from East Asia alone increased the EASM strength by almost 5%. Considering the effect of the westward shift of WPSH, the dipole changes in emissions together increased the EASM by 5%-15% during 2013-17, revealing an important role of South Asian aerosols in changing the East Asian climate.

The direct perturbation of anthropogenic aerosols on Earth's energy balance [i.e., direct aerosol radiative forcing (DARF)] remains uncertain in climate models. In this study, we investigate the uncertainty of DARF associated with aerosol vertical distribution, using simulation results from 14 global models within phase 6 of the Coupled Model Intercomparison Project (CMIP6). The column mass loading for each aerosol species is first normalized to the multimodel average for each model, which is called the mass-normalization process. The unified radiative transfer model and aerosol optical parameter are used, so that the differences in the calculated DARF are solely attributed to the difference in aerosol vertical profiles. The global mean DARF values in 2014 with respect to 1850 before and after mass normalization are -0.77 +/- 0.52 and -0.81 +/- 0.12 W m(-2) respectively, assuming external mixing, which indicates that the intermodel difference in aerosol vertical distribution accounts for similar to 20% of the total DARF uncertainty. We further conduct two separate experiments by normalizing aerosol optical depth (AOD) and aerosol single scattering albedo (SSA) profiles, respectively, and find that the vertical distribution of SSA results in larger DARF uncertainty (0.17 W m(-2)) than that of AOD (0.10 W m(-2)). Finally, compared with CALIPSO observation, CMIP6 models tend to produce higher aerosol layers. The bias in modeled aerosol profile with respect to CALIPSO leads to stronger DARF, especially for land regions.

Recent increases in surface temperature and snow melt acceleration in the Himalayan region are influenced by many factors. Here we investigate the influence of absorbing aerosols, including black carbon and dust, on surface temperature and snow melt in western, central, and eastern parts of the India-Nepal Himalayan region (INHR). We compare 40-y simulations (1971-2010) one with all evolving forcing agents representative of a present-day aerosol scenario, compared to a low aerosol forcing scenario. The difference between these scenarios shows a significant increase in surface air temperature, with higher warming in parts of Western and Central Himalaya (-0.2-2 degrees C) in the months of April and May. Higher absorbing aerosol (BC and dust abundance) both at the surface and in the atmospheric column, in the present-day aerosol simulations, led to increases in atmospheric radiative forcing and surface shortwave heating rate forcing (SWHRF), compared to the low aerosol forcing case. Therefore, the absorbing aerosols cause anomalous atmospheric heat energy transfer to land due to high surface SWHRF and changes in surface energy flux, leading to snow melt. The present model version did not parameterize snow albedo feedback, which would increase the magnitudes of the changes simulated here. (C) 2021 Elsevier B.V. All rights reserved.

Studies of the climate effects of black carbon (BC) in East Asia are not abundant and the effects remain uncertain. Using the Community Earth System Model version 1 (CESM1) with Peking University's emissions data, the fast response of the atmospheric water cycle to anthropogenic BC during summer in East Asia is investigated in this study. Results show that the CESM1-simulated BC concentration and its direct effective radiative forcing are comparable to observations. With the combination of aerosol-radiation interaction (ARI) and non-aerosol-radiation interaction (including aerosol-cloud interaction and surface albedo effects), anthropogenic BC induces a wetter south and drier north pattern over East Asia during summer. Also, anthropogenic BC affects the summer precipitation primarily through changing moisture transport rather than altering local evaporation over East Asia. Using the self-developed atmospheric water tracer method, the responses of dominant moisture sources [the tropical Indian Ocean (TIO) and northwest Pacific] to anthropogenic BC are investigated. Results show that the moisture originating from southwest monsoon-related sources (especially the TIO) is more responsive to anthropogenic BC effects over East Asia. In particular, differing from total precipitation, TIO-supplied precipitation shows a significant response to the ARI of anthropogenic BC over East Asia. Process analyses show that anthropogenic BC affects the southwest monsoon-related moisture supplies primarily via advection, deep convection, and cloud macrophysics. Interestingly, the anthropogenic BC-induced changes of TIO-supplied water vapor in these three processes are all dominated by the ARI over East Asia.

Black carbon (BC) aerosol is a significant and short-lived climate forcing factor. Here, the direct effects of BC emissions from India (IDBC) and China (CNBC) are investigated in East Asia during summer using the state-of-the-art regional climate model RegCM4. In summer, IDBC and CNBC account for approximately 30% and 46% of the total BC emissions in Asia, respectively. The total BC column burden from the two countries and corresponding TOA effective radiative forcing are 1.58 mg m(-2) and +1.87 W m(-2) in East Asia, respectively. The regional air temperature increases over 0.3 K at maximum and precipitation decreases 0.028 mm day(-1) on average. Individually, IDBC and CNBC each can bring about rather different effects on regional climate. IDBC can result in a cooling perturbation accompanied by a substantially increased cloud amount and scattering aerosol loading, resulting in a complex response in the regional precipitation, while CNBC can lead to regional warming, and further induce a local flood in northern China or drought in southern China depending on the opposite but significant circulation anomalies. CNBC plays a dominant role in modulating the regional climate over East Asia due to its higher magnitude, wider coverage, and stronger climate feedback. The direct effect of the total BC from both countries is not a linear combination of that of IDBC and CNBC individually, suggesting that the regional climate responses are highly nonlinear to the emission intensity or aerosol loading, which may be greatly related to the influences of the perturbed atmospheric circulations and climate feedback.

We use Aerosol Robotic Network (AERONET) observation data to empirically determine how natural and anthropogenic aerosol categories (i.e. mineral dust, biomass burning, and urban-industrial aerosols) affect light extinction, showing that their radiative forcing varies strongly with the surface albedo. Generally, the radiative forcing depends on the aerosol loading, but the efficiency varies with the aerosol type and aerosol-radiation-surface interactions. Desert dust, biomass burning and urban-industrial aerosols can exhibit dramatic shifts in radiative forcing at the top of the atmosphere, from cooling to warming, at surface albedos from below 0.5 to above 0.75. Based on the linear relationship between the radiative forcing efficiency and surface albedo for aeolian aerosols, using Moderate Resolution Imaging Spectroradiometer (MODIS) AOT (Aerosol Optical Thickness) and surface albedo data, we characterized a large Asian dust event during the spring of 2001, and demonstrate its immense spatially varying radiative forcing, ranging from about -84.0 to +69.3 W/m(2). For extensive Russian wildfires during the summer of 2010, strong radiative cooling forcing variability of biomass combustion aerosols is found, ranging from about -86.3 to +3.1 W/m(2). For a thick urban-industrial aerosol haze over northern India during the winter of 2017, a large range of about -85.0 to -0.3 W/m(2) is found. These wide ranges underscore the need to accurately define aerosol-radiation-surface interactions.

In order to describe the means, variability and trends of the aerosol radiative effects on the southwest Atlantic coast of Europe, 11 years of aerosol light scattering (sigma(sp)) and 4 years of aerosol light absorption (sigma(sp)) are analyzed. A 2006-2016 trend analysis of sigma(sp) for D < 10 mu m indicates statistically significant trends for March, May-June and September-November, with a decreasing trend ranging from -1.5 to - 2.8 Mm(-1)/year. In the 2009-2016 period, the decreasing trend is only observed for the months of June and September. For scattering Angstrom exponent (SAE) there is an increasing trend during June with a rate of 0.059/year and a decreasing trend during October with - 0.060/year. The trends observed may be caused by a reduction of Saharan dust aerosol or a drop in particle loading in anthropogenic influenced air masses. The relationship between SAE and absorption Angstrom exponent is used to assess the aerosol typing. Based on this typing, the sub-micron particles are dominated by black carbon, mixed black and brown carbon or marine with anthropogenic influences, while the super-micrometer particles are desert dust and sea spray aerosol. The mean and standard deviation of the dry aerosol direct radiative effect at the top of the atmosphere (DRETOA) are -4.7 +/- 4.2 W m(-2). DRETOA for marine aerosol shows all observations more negative than - 4 W m(-2 )and for anthropogenic aerosol type, DRETOA ranges from -5.0 to -13.0 W m(-2). DRETOA of regional marine aerosol ranges from -3 to -7 W m(-2), as it consists of a mixture of sea salt and anthropogenic aerosol. The variability in DRETOA is mainly dependent on AOD, given that variations in backscatter fraction and the single scattering albedo tend to counteract each other in the radiative forcing efficiency equation. The results shown here may help in interpretation of satellite retrieval products and provide context for model evaluation.

Black carbon aerosol (BC) has a significant influence on regional climate changes because of its warming effect. Such changes will feed back to BC loadings. Here, the interactions between the BC warming effect and the East Asian monsoon (EAM) in both winter (EAWM) and summer (EASM) are investigated using a regional climate model, RegCM4, that essentially captures the EAM features and the BC variations in China. The seasonal mean BC optical depth is 0.021 over East Asia during winter, which is 10.5% higher than that during summer. Nevertheless, the BC direct radiative forcing is 32% stronger during summer (+1.85 W m(-2)). The BC direct effect would induce lower air to warm by 0.11-0.12 K, which causes a meridional circulation anomaly associated with a cyclone at 20 degrees-30 degrees N and southerly anomalies at 850 hPa over East Asia. Consequently, the EAM circulation is weakened during winter but enhanced during summer. Precipitation is likely increased, especially in southern China during summer (by 3.73%). Relative to BC changes that result from EAM interannual variations, BC changes from its warming effect are as important but are weaker. BC surface concentrations are decreased by 1%-3% during both winter and summer, whereas the columnar BC is increased in south China during winter. During the strongest monsoon years, the BC loadings are higher at lower latitudes than those during the weakest years, resulting in more southerly meridional circulation anomalies and BC feedbacks during both winter and summer. However, the interactions between the BC warming effect and EAWM/EASM are more intense during the weakest monsoon years.

The large uncertainty in estimating the global aerosol radiative forcing (ARF) is one of the major challenges the climate community faces for climate projection. While the global-mean ARF may affect global quantities such as surface temperature, its spatial distribution may result in local thermodynamical and, thus, dynamical changes. Future changes in aerosol emissions distribution could further modulate the atmospheric circulation. Here, the effects of the spatial distribution of the direct anthropogenic ARF are studied using an idealized global circulation model, forced by a range of estimated-ARF amplitudes, based on the Copernicus Atmosphere Monitoring Service data. The spatial distribution of the estimated-ARF is globally decomposed, and the effects of the different modes on the circulation are studied. The most dominant spatial distribution feature is the cooling of the Northern Hemisphere in comparison to the Southern Hemisphere. This induces a negative meridional temperature gradient around the equator, which modulates the mean fields in the tropics. The ITCZ weakens and shifts southward, and the Northern (Southern) Hemisphere Hadley cell strengthens (weakens). The localization of the ARF in the Northern Hemisphere midlatitudes shifts the subtropical jet poleward and strengthens both the eddy-driven jet and Ferrel cell, because of the weakening of high-latitude eddy fluxes. Finally, the larger aerosol concentration in Asia compared to North America results in an equatorial superrotating jet. Understanding the effects of the different modes on the general circulation may help elucidate the circulation's future response to the projected changes in ARF distribution.