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A comprehensive global investigation on the impact of reduction (changes) in aerosol emissions due to Coronavirus disease-2019 (COVID-19) lockdowns on aerosol single scattering albedo (SSA) utilizing satellite observations and model simulations is conducted for the first time. The absolute change in Ozone Monitoring Instrument (OMI) retrieved, and two highly-spatially resolved models (Modern-Era Retrospective Analysis for Research and Applications-2 (MERRA-2) and Copernicus Atmosphere Monitoring Service (CAMS)) simulated SSA is <4% (<0.04-0.05) globally during COVID (2020) compared to normal (2015-2019) period. Change in SSA during COVID is not significantly different from long-term and year-to-year variability in SSA. A small change in SSA indicates that significant reduction in anthropogenic aerosol emissions during COVID-19 induced lockdowns has a negligible effect in changing the net contribution of aerosol scattering and/or absorption to total aerosol extinction. The changes in species-wise aerosol optical depth (AOD) are examined in detail to explain the observed changes in SSA. Model simulations show that total AOD decreased during COVID-19 lockdowns, consistent with satellite observations. The respective contributions of sulfate and black carbon (BC) to total AOD increased, which resulted in a negligible change in SSA during the spring and summer seasons of COVID over South Asia. Europe and North America experience a small increase in SSA (<2%) during the summer season of COVID due to a decrease in BC contribution. The change in SSA (2%) is the same for a small change in BC AOD contribution (3%), and for a significant change in sulfate AOD contribution (20%) to total AOD. Since, BC SSA is 5-times lower (higher absorption) than that of sulfate SSA, the change in SSA remains the same. For a significant change in SSA to occur, the BC AOD contribution needs to be changed significantly (4-5 times) compared to other aerosol species. A sensitivity analysis reveals that change in aerosol radiative forcing during COVID is primarily dependent on change in AOD rather than SSA. These quantitative findings can be useful to devise more suitable future global and regional mitigation strategies aimed at regulating aerosol emissions to reduce environmental impacts, air pollution, and public health risks.

期刊论文 2024-09-15 DOI: 10.1016/j.atmosenv.2024.120649 ISSN: 1352-2310

The Tibetan Plateau holds the largest mass of snow and ice outside of the polar regions. The deposition of light-absorbing particles (LAPs) including mineral dust, black carbon and organic carbon and the resulting positive radiative forcing on snow (RFSLAPs) substantially contributes to glacier retreat. Yet how anthropogenic pollutant emissions affect Himalayan RFSLAPs through transboundary transport is currently not well known. The COVID-19 lockdown, resulting in a dramatic decline in human activities, offers a unique test to understand the transboundary mechanisms of RFSLAPs. This study employs multiple satellite data from the moderate resolution imaging spectroradiometer and ozone monitoring instrument, as well as a coupled atmosphere-chemistry-snow model, to reveal the high spatial heterogeneities in anthropogenic emissions-induced RFSLAPs across the Himalaya during the Indian lockdown in 2020. Our results show that the reduced anthropogenic pollutant emissions during the Indian lockdown were responsible for 71.6% of the reduction in RFSLAPs on the Himalaya in April 2020 compared to the same period in 2019. The contributions of the Indian lockdown-induced human emission reduction to the RFSLAPs decrease in the western, central, and eastern Himalayas were 46.8%, 81.1%, and 110.5%, respectively. The reduced RFSLAPs might have led to 27 Mt reduction in ice and snow melt over the Himalaya in April 2020. Our findings allude to the potential for mitigating rapid glacial threats by reducing anthropogenic pollutant emissions from economic activities.

期刊论文 2023-05-31 DOI: 10.1093/pnasnexus/pgad172

Coronavirus disease (COVID-19) has disrupted health, economy, and society globally. Thus, many countries, including China, have adopted lockdowns to prevent the epidemic, which has limited human activities while affecting air quality. These affects have received attention from academics, but very few studies have focused on western China, with a lack of comparative studies across lockdown periods. Accordingly, this study examines the effects of lockdowns on air quality and pollution, using the hourly and daily air monitoring data collected from Lanzhou, a large city in Northwest China. The results indicate an overall improvement in air quality during the three lockdowns compared to the average air quality in the recent years, as well as reduced PM2.5, PM10, SO2, NO2, and CO concentrations with different rates and increased O3 concentration. During lockdowns, Lanzhou's morning peak of air pollution was alleviated, while the spatial characteristics remained unchanged. Further, ordered multi-classification logistic regression models to explore the mechanisms by which socioeconomic backgrounds and epidemic circumstances influence air quality revealed that the increment in population density significantly aggravated air pollution, while the presence of new cases in Lanzhou, and medium- and high-risk areas in the given district or county both increase the likelihood of air quality improvement in different degrees. These findings contribute to the understanding of the impact of lockdown on air quality, and propose policy suggestions to control air pollution and achieve green development in the post-epidemic era.

期刊论文 2023-05-01 DOI: http://dx.doi.org/10.1016/j.uclim.2023.101533 ISSN: 2212-0955

The COVID-19 lockdown restrictions influenced global atmospheric aerosols. We report aerosol variations over India using multiple remote sensing datasets [Moderate Resolution Imaging Spectroradiometer (MODIS), Ozone Monitoring Instrument (OMI), Cloud-Aerosol Lidar, and Infrared Pathfinder (CALIPSO)], and model reanalysis [Copernicus Atmosphere Monitoring Service (CAMS)] during the lockdown implemented during the COVID-19 pandemic outbreak period from March 25 to April 14, 2020. Our analysis shows that, during this period, MODIS and CALIPSO showed a 30-40% reduction in aerosol optical depth (AOD) over the Indo-Gangetic Plain (IGP) with respect to decadal climatology (2010-2019). The absorbing aerosol index and dust optical depth measurements also showed a notable reduction over the Indian region, highlighting less emission of anthropogenic dust and also a reduced dust transport from West Asia during the lockdown period. On the contrary, central India showed an similar to 12% AOD enhancement. CALIPSO measurements revealed that this increase was due to transported biomass burning aerosols. Analysis of MODIS fire data product and CAMS fire fluxes (black carbon, SO2, organic carbon, and nitrates) showed intense fire activity all over India but densely clustered over central India. Thus, we show that the lockdown restrictions implemented at the government level have significantly improved the air quality over northern India but fires offset its effects over central India. The biomass-burning aerosols formed a layer near 2-4 km (AOD 0.08-0.1) that produced heating at 3-4 K/day and a consequent negative radiative forcing at the surface of similar to-65 W/m(2) (+/- 40 W/m(2)) over the central Indian region.

期刊论文 2021-09-20 DOI: 10.3389/fenvs.2021.746090
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