Carbonaceous particles are an important radiative forcing agent in the atmosphere, with large temporal and spatial variations in their concentrations and compositions, especially in remote regions. This study reported the delta C-14 and delta C-13 of total carbon (TC) and water-insoluble particulate carbon (IPC) of the total suspended particles (TSP) and PM2.5 at a remote site of the eastern Tibetan Plateau (TP), a region that is influenced by heavy air pollution from Southwest China. The average organic carbon and elemental carbon concentrations of TSP samples in this study were 3.20 +/- 2.38 mu g m(-3) and 0.68 +/- 0.67 mu g m(-3), respectively, with low and high values in summer and winter, respectively. The fossil fuel contributions of TC in TSP and PM2.5 samples were 18.91 +/- 7.22% and 23.13 +/- 12.52%, respectively, both of which were far lower than that in Southwest China, indicating the importance of non-fossil contributions from local sources. The delta C-13 of TC in TSP samples of the study site was -27.06 +/- 0.96 parts per thousand, which is between the values of long-range transported sources (e.g., Southwest China) and local biomass combustion emissions. Therefore, despite the contribution from the long-range transport of particles, aerosols emitted from local biomass combustion also have an important influence on carbonaceous particles at the study site. The findings of this work can be applied to other remote sites on the eastern TP and should be considered in related research in the future.

Carbonaceous particles are an important radiative forcing agent in the atmosphere, with large temporal and spatial variations in their concentrations and compositions, especially in remote regions. This study reported the delta C-14 and delta C-13 of total carbon (TC) and water-insoluble particulate carbon (IPC) of the total suspended particles (TSP) and PM2.5 at a remote site of the eastern Tibetan Plateau (TP), a region that is influenced by heavy air pollution from Southwest China. The average organic carbon and elemental carbon concentrations of TSP samples in this study were 3.20 +/- 2.38 mu g m(-3) and 0.68 +/- 0.67 mu g m(-3), respectively, with low and high values in summer and winter, respectively. The fossil fuel contributions of TC in TSP and PM2.5 samples were 18.91 +/- 7.22% and 23.13 +/- 12.52%, respectively, both of which were far lower than that in Southwest China, indicating the importance of non-fossil contributions from local sources. The delta C-13 of TC in TSP samples of the study site was -27.06 +/- 0.96 parts per thousand, which is between the values of long-range transported sources (e.g., Southwest China) and local biomass combustion emissions. Therefore, despite the contribution from the long-range transport of particles, aerosols emitted from local biomass combustion also have an important influence on carbonaceous particles at the study site. The findings of this work can be applied to other remote sites on the eastern TP and should be considered in related research in the future.

Based on glacio-meteorological records, 7 years of in-situ mass balance data, and a temperature-index model, the long-term annual and seasonal mass balances of Shiyi Glacier in the northeast Tibetan Plateau (TP) were reconstructed from 1963/64 to 2016/17. Variations were then linked to local climatic and macroscale circulation changes. The model was calibrated based on in-situ mass balance data and was driven by daily air temperature and precipitation data recorded at nearby alpine meteorological stations. The results show that the reconstructed annual mass balance experienced an overall downward trend over the past 54 years, with a remarkably high mass loss rate during 1990/91-2016/17. Analysis of mass balance sensitivity and local climatic changes shows that the pronounced mass loss since the 1990s can be mainly attributed to cumulative positive temperature increases caused by air temperature increases and prolongation of the ablation season. From the perspective of macroscale circulation, the reconstructed annual mass balance values correlate well with zonal wind speeds (June to September) in the glacierized region. For the positive/negative phase of the annual mass balance, an inverse spatial pattern in relation to geopotential height change (low/high-pressure centres) and corresponding conversion of cyclonic/anti-cyclonic circulation were present in northern hemisphere mid-latitudes. Comparative analysis of existing long-term mass balance series over the TP indicates that asynchronous climatic changes in the different glacierized regions led to inconsistent interannual fluctuations in glacier mass balance.