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The Pan-Third Pole contains the largest number of glaciers outside the polar region that plays a crucial role in atmospheric circulation and the hydrological cycle. However, this pristine region has undergone rapid change through complex interactions including the black carbon (BC) enhanced warming effect and glacier melting. Study shows, Weather Research and Forecasting coupled with Chemistry (WRF-Chem) simulation is able to capture distinctive seasonal variability of BC. The result from our sensitivity experiments revealed that South Asia (SA; 60.7%) and East Asia (EA; 32.9%) contributed more toward the Tibetan Plateau (TP). Our analysis on aerosol-boundary feedback interaction revealed BC expand planetary boundary layer height by 5.0% and 4.8% over SA and EA, respectively, which facilitates BC dispersion and transportation. Whereas, we also found that under the influence of different wind regimes the significant BC transport flux aloft over the TP and the upper troposphere and lower stratosphere. Additionally, mountain-valley channel and synoptic and local meteorological processes also facilitated BC transport to the TP. This study also evaluated the effect of BC on direct radiative forcing and calculated subsequent temperature changes. A strong dimming effect of BC corroborated with the following negative surface temperature changes. However, enhanced BC concentration during winter and spring caused the increase in temperature over the TP. Here, the WRF-Chem model, synergy on aerosol-boundary feedback, BC transport flux, and source-receptor methods confirmed the significant BC contribution and transportation, and notable BC-induced warming over TP. Such trans-Himalayan BC transport and associated warming could grim glacier melt and water availability in the region.

期刊论文 2022-03-27 DOI: 10.1029/2021JD035772 ISSN: 2169-897X

The Pan-Third Pole contains the largest number of glaciers outside the polar region that plays a crucial role in atmospheric circulation and the hydrological cycle. However, this pristine region has undergone rapid change through complex interactions including the black carbon (BC) enhanced warming effect and glacier melting. Study shows, Weather Research and Forecasting coupled with Chemistry (WRF-Chem) simulation is able to capture distinctive seasonal variability of BC. The result from our sensitivity experiments revealed that South Asia (SA; 60.7%) and East Asia (EA; 32.9%) contributed more toward the Tibetan Plateau (TP). Our analysis on aerosol-boundary feedback interaction revealed BC expand planetary boundary layer height by 5.0% and 4.8% over SA and EA, respectively, which facilitates BC dispersion and transportation. Whereas, we also found that under the influence of different wind regimes the significant BC transport flux aloft over the TP and the upper troposphere and lower stratosphere. Additionally, mountain-valley channel and synoptic and local meteorological processes also facilitated BC transport to the TP. This study also evaluated the effect of BC on direct radiative forcing and calculated subsequent temperature changes. A strong dimming effect of BC corroborated with the following negative surface temperature changes. However, enhanced BC concentration during winter and spring caused the increase in temperature over the TP. Here, the WRF-Chem model, synergy on aerosol-boundary feedback, BC transport flux, and source-receptor methods confirmed the significant BC contribution and transportation, and notable BC-induced warming over TP. Such trans-Himalayan BC transport and associated warming could grim glacier melt and water availability in the region.

期刊论文 2021-08-01 DOI: http://dx.doi.org/10.1029/2021JD035772 ISSN: 2169-897X

The Pan-Third Pole (PTP), stretching from Eastern Asia to Middle-central Europe, has experienced unprecedented accelerated warming and even retreat of glaciers. Absorbing aerosols reduce snow and ice albedo and radiative forcing, consequently enhancing a great melting of snow cover and ice sheet in the PTP. Employing the 10-year (2007-2016) space-based active and passive measurements, this study investigated the distribution, optical properties and decadal trends for dominating aerosols at a seasonal scale in the PTP divided into six subregions. Results showed that the sub-regions of PTP were mainly dominated by dust, polluted dust and elevated smoke. The Taklimakan Desert (TD) and the Iranian Plateau (IP) were dominated by mineral dust, accounting for 96% and 86% of the total aerosol extinction while the Central Europe (CE), Indo-China (IC) and Anatolia Plateau (AP) were dominated by the mixture of the dominating aerosol types. The mean aerosol extinction coefficient (MAEC) showed an obvious variability depending on the sub-regions and a tendency of decreasing with an increase in the topographic height. The strongest extinction layer (>0.1 km(-1)) mainly occurred below 4 km and the weak extinction layers (>0.001 km(-1)) were mainly distributed between 5 km and 8 km, indicating pronounced vertical transport in the region. The decadal trends of columnar aerosol optical depth (AOD) showed a relation with the contributions of the dominating aerosol types. For example, significant upward or downward trends of total aerosol loading in the IC region were driven by elevated smoke while the AOD trends of total aerosol loading for the CE, the AP and the IP were driven by the dominating aerosol types. The Tibetan Plateau (TP), the cleanest region in the PTP, has been regularly exposed to polluted air masses with significant amounts of absorbing aerosols. Therefore, understanding the dominating aerosol types, properties and decadal trends in the PTP region will contribute considerably to assessing their effects on radiative forcing, climate change, and even snowmelt and glacier retreat.

期刊论文 2020-10-15 DOI: 10.1016/j.atmosenv.2020.117738 ISSN: 1352-2310
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