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Remote region is normally considered a receptor of long-range transported pollutants. Monitoring stations are important platforms for investigating the atmospheric environment of remote regions. However, the potential contribution of very local sources around these stations may produce important influences on its atmospheric environment, which is still barely studied. In this study, major ions of precipitation were investigated simultaneously at a typical remote station (Nam Co station) and other sites nearby on the Tibetan Plateau (TP) - the so-called The Third Pole in the world. The results showed that despite low values compared to those of other remote regions, the concentrations of major ions in precipitation of Nam Co station (e.g., Ca2+: 32.71 mu eq/L; SO42- : 1.73 mu eq/L) were significantly higher than those at a site around 2.2 Km away ( Ca2+: 11.47 mu eq/L; SO42- : 0.64 mu eq/L). This provides direct evidence that atmospheric environment at Nam Co station is significantly influenced by mineral dust and pollutants emitted from surface soil and anthropogenic pollutants of the station itself. Therefore, numbers of other related data reported on the station are influenced. For example, the aerosol concentration and some anthropogenic pollutants reported on Nam Co station should be overestimated. Meanwhile, it is suggested that it is cautious in selecting sites for monitoring the atmospheric environment at the remote station to reduce the potential influence from local sources.

期刊论文 2023-12-01 DOI: http://dx.doi.org/10.1007/s10661-023-12113-9 ISSN: 0167-6369

The quantitative and qualitative characterization of ions and inorganic nitrogen in precipitation assists in understanding the accompanying sources and chemistry of regional precipitation. A total of 212 event-based precipitation samples were collected from four sites in Bangladesh in 2017 to investigate the physicochemical characteristics, sources, and deposition of atmospheric ionic constituents and inorganic nitrogen. During the entire monitoring period, 5.7% of the total samples were acidic (i.e., pH Cox's Bazar > Dinajpur > Sylhet, whereas the anthropogenic species exhibited the order of Dinajpur > Satkhira > Sylhet > Cox's Bazar, underlining the local and regional impacts of these species in Bangladesh. Based on the source apportionment, the sources were categorized as marine (Na+ and Cl-), terrigenous (Ca2+, Mg2+, and HCO3-), fossil fuel combustion (NO3- and SO42-), agriculture (NH4+), and biomass burning (K+). The Cl- in Sylhet and Satkhira suggests additional sources associated with anthropogenic activities. The back-trajectory analyses and the National Centers for Environmental Prediction's final (NCEP FNL) datasets illustrate the presence of significantly diverse air masses with contributions from various sources in the monsoon and non-monsoon climates. Both the amount of precipitation and the ionic quantity governs the fluxes in Bangladesh. The Na+ % and SAR lie under the safe category suggesting a good precipitation water quality for agriculture and soil in Bangladesh, while the deposition of inorganic nitrogen has resulted in a value above the threshold line (10 kg ha(-1) y(-1)). Thus, this study conveys a comprehensive picture of the ionic composition, providing a baseline dataset to assess the atmospheric environment in this lowland region.

期刊论文 2021-02-20 DOI: http://dx.doi.org/10.1016/j.atmosres.2020.105414 ISSN: 0169-8095
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