Use of forest biomass may induce changes in the aerosol emissions, with subsequent impacts on the direct and indirect climate effects of these short-lived climate forcers. We studied how alternative wood use scenarios affected the aerosol emissions and consequent radiative forcing in Finland. In all alternative scenarios, the harvest level of forest biomass was increased by 10 million m3 compared to the baseline. The increased biomass harvest was assigned to four different uses: (i) to sawn wood, (ii) to pulp-based products, (iii) to energy biomass combusted in small-scale appliances or (iv) to energy biomass combusted in medium-to-large scale boilers. Aerosol emissions (black carbon (BC), organic carbon (OC) and sulphur dioxide (SO2)) under these scenarios were estimated using displacement factors (DFs). The global aerosol-climate model ECHAM-HAMMOZ was used to study instantaneous radiative forcing due to aerosol-radiation interactions (IRFARI) and effective radiative forcing (ERF), based on the differences in aerosol emissions between the alternative wood use scenarios and the baseline scenario. The results indicated that the use of sawn wood and energy biomass combusted in medium- to large-scale boilers decreased radiative forcings, implying climate cooling, whereas the increased use of pulpwood increased them. Energy biomass combustion in small-scale appliances increased IRFARI by 0.004 W m-2 but decreased ERF by -0.260 W m-2, specifically due to a strong increase in carbonaceous aerosols. Alternative use of forest biomass notably influenced aerosol emissions and their climate impacts, and it can be concluded that increased forest biomass use requires a comprehensive assessment of aerosol emissions alongside greenhouse gases (GHGs). Given the consequent reduction in radiative forcing from aerosol emissions, we conclude that the greatest overall climate benefits could be achieved by prioritising the production of long-lived wood-based products.

There has been growing interest in the potential of short-lived climate forcer (SLCF) mitigation to reduce near-term global warming. Black carbon (BC), organic carbon (OC), and sulfur dioxide (SO2) are SLCFs which change the Earth's radiative balance directly by affecting radiation, and indirectly by altering cloud properties. We used the ECHAM-HAMMOZ aerosol-climate model to study the radiative forcings due to mitigating the anthropogenic emissions of BC, OC, and SO2 from Chile and Mexico. Limiting our analysis to areas where these emissions had notable effects on both aerosol and clouds, we found that the total radiative forcings of anthropogenic aerosol emissions are different for Chile and Mexico. This was explained by differences in aerosol emissions, orography, and meteorology in these two countries. Especially the radiative forcing for Chilean emissions was influenced by the persistent stratocumulus cloud deck west of Chile. To reduce the uncertainty of our radiative forcing calculations, we nudged the wind and surface pressure toward pre-generated fields. As nudging affects the calculated effective radiative forcing (ERF), we here used the identifier ERFNDG. Our results indicate that the removal of OC and SO2 emissions caused a positive ERFNDG while the removal of BC emissions caused a positive ERFNDG for Chile, but a negative ERFNDG for Mexico. When accounting for co-emission of other aerosol compounds, reducing BC emissions led to positive ERFNDG in both countries. Compared to China, the removal of anthropogenic SO2 emissions in Chile and Mexico caused a much larger global average ERFNDG per emitted unit mass of SO2.

Diesel vehicles are a significant source of black carbon (BC) and ozone precursors, which are important contributors to climate warming, degrade air quality and harm human health. Reducing diesel emissions could mitigate near-term climate change with significant co-benefits. This study quantifies the global and regional climate impacts of BC and co-emitted short-lived climate forcers (SLCFs) from present-day on-road diesel vehicles, as well as future impacts following a current legislation emission scenario. Atmospheric concentrations are calculated by the chemical transport model OsloCTM2. The following radiative forcing (RF) and equilibrium surface temperature responses are estimated. For year 2010 on-road diesel emissions we estimate a global-mean direct RF from BC of 44 m W/m(2) and an equilibrium surface temperature response of 59 mK, including the impact of BC deposition on snow. Accounting for cooling and warming impacts of co-emitted SLCFs results in a net global-mean RF and warming of 28 mW/m(2) and 48 mK, respectively. Using the concept of Regional Temperature change Potential (RIP), we find significant geographical differences in the responses to regional emissions. Accounting for the vertical sensitivities of the forcing/response relation amplifies these differences. In terms of individual source regions, emissions in Europe give the largest regional contribution to equilibrium warming caused by year 2010 on-road diesel BC, while Russia is most important for Arctic warming per unit emission. The largest contribution to warming caused by the year 2050 on-road diesel sector is from emissions in South Asia, followed by East Asia and the Middle East. Hence, in regions where current legislation is not sufficient to outweigh the expected growth in activity, accelerated policy implementation is important for further future mitigation. (C) 2014 Elsevier Ltd. All rights reserved.