To provide insight into dust sources in snow deposited during the non-monsoon period on the Tibetan Plateau, detailed post-Archean Australian shale (PAAS)-normalized rare earth element (REE) distribution patterns and variations in REE tracers, such as La/Yb, La/Er, and Gd/Yb with depth, as well as the distribution of samples in the plots of REE ratio pairs, such as La/Yb vs. Y/sigma REE, La/Er vs. Gd/Er, and Y/La vs. Nd/Er, were compared in seven potential dust source areas in Asia. Snow samples from five glaciers, i.e., Qiumianleike (QMLK), Meikuang (MK), Yuzhufeng (YZF), Xiaodongkemadi (XDKMD), and Gurenhekou (GRHK), were collected from April 26 to May 13 before the onset of monsoon activity. The results show that dust trapped in snow pits from the studied glaciers, i.e., QMLK, MK, XDKMD, and GRHK, has varying degrees of contribution from the Taklimakan Desert, Qaidam Basin, and the surface soil of the Tibetan Plateau. There are signals of the Tengger and Badain Jaran Desert and Chinese Loess in the MK and XDKMD snow pit samples or in the QMLK and GRHK surface samples from the REE tracers; however, from the point of view of the land location, the three dust sources should not be the major contributors. Signals of dust from the Indian Thar Desert were occasionally detected from the MK, YZF, and XDKMD snow pit samples and GRHK surface snow samples, implying the intrusion of early Indian monsoon activities to the sites. The dust signal from the Thar Desert in India from the YZF glacier is significantly greater than that from the XDKMD and MK glaciers. These findings were also supported by the tracer of dust transmitted to the three snow pits through the air mass backward trajectories. The new finding of this study is that dust from the Indian Desert can even reach the Kunlun Mountains in the northern region of the Tibetan Plateau. The conclusions are helpful in interpreting the sources of dust and the pollutants absorbed by dust particles, as well as the extent of the impact of Indian monsoon activities at the end of the non-monsoon season on the plateau.
In order to determine the current levels, spatial distribution patterns, and potential pollution of trace elements (TEs) in the atmosphere of the Tibetan Plateau (TP), snow pit samples were collected in May 2016 from five TP glaciers: Qiyi (QY), Hariqin (HRQ), Meikuang (MK), Yuzhufeng (YZF), and Xiao-dongkemadi (XDKMD). Concentrations of 13 TEs (Al, Ba, Cd, Co, Cr, Cu, Fe, Li, Pb, Sb, Sr, U, and Zn) in the snow were measured. The spatial distribution patterns and depth profiles of TEs from the studies sites revealed that the influence of dust on TEs was more significant on the MK and YZF glaciers than on the QY, HRQ, and XDKMD glaciers. The spatial distributions of TE EFFe values differed from their concentrations, however. The enrichment factor (EF) values and concentrations of some TEs in the YZF, QY, and XDKMD glaciers revealed that the pollution levels of these elements were significantly lower than those found in previous research. Examination based on EFs, principal component analysis, as well as the calculated non-dust contributions of TEs, revealed that dust was the principal source for most TEs in all five glaciers, while biomass burning was another potential natural source for TEs in some glaciers, such as QY. In contrast, Cd, Ba, Sr, Cu, Pb, Zn, and Sb were occasionally affected by anthropogenic sources such as road traffic emissions, fossil fuel combustion, and mining and smelting of nonferrous metals in and beyond the TP. Air mass backward trajectories revealed that potential pollutants were transported not only from local sources but also from Xinjiang Province in northwestern China, as well as South Asia, Central Asia, the Middle East, and Europe. (c) 2020 Elsevier Ltd. All rights reserved.