Atmospheric aerosols have important impacts on global radiative forcing, air pollution, and human health. This study investigated the optical and physical properties of aerosol layers over Australia from 2007 to 2019 using the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) Level 2 aerosol products. Australia was divided into three sub-regions (western highlands, central plains, and eastern ranges). Interannual and seasonal optical property variations in aerosol layers in the three sub-regions were analyzed and compared. Results showed that annual mean values of AOD(L) (lowest aerosol layer AOD) and AOD(T) (total AOD of all aerosol layers) were always higher in the eastern ranges region than the other two regions from 2007 to 2019. The reason could be that Australian population was predominantly located in the eastern ranges region, where more human activities could bring significant aerosol loadings. B-L (base height of the lowest aerosol layer), H-L (top height of the lowest aerosol layer), and H-H (top height of the highest aerosol layer) all showed trends of western highlands > eastern mountains > central plains, indicating that the higher the elevation, the higher the B-L, H-L, and H-H. T-L (thickness of the lowest aerosol layer) was higher during the day than at night, which might account for increased diurnal atmospheric convection and nocturnal aerosol deposition. DRL (depolarization ratio of the lowest aerosol layer) was higher in the western highlands and central plains than the eastern mountains, probably because these two regions have large deserts with more irregularly shaped dust aerosols. CRL (color ratio of the lowest aerosol layer) had slightly higher values in the eastern ranges than the other two regions, probably due to the wet climate of the eastern ranges, where aerosols were more hygroscopic and had larger particle sizes. This study can provide technical support for the control and management of regional air pollutants.
Mineral dust aerosols over the Himalayas are assessed using polarization-resolved observations of Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite over 11 years (2006-2018). The extinction coefficient due to dust aerosols is retrieved using observations of the depolarization ratio which gives the relative contribution of dust aerosols in the scattering volume. Dust extinction coefficients show significant regional and seasonal variation over the Himalayas. High dust loading is observed during the pre-monsoon season (March-May) whereas dust loading is low during the summer monsoon season (June-September). This is due to the reduced dust transport associated with the weak westerlies that prevailed over the Himalayas. Regionally, the mid-Himalayas is characterized by the highest dust extinction coefficient with a 10-fold increase as the season changes from winter (December-February) to pre-monsoon (March-May). Polluted dust (dust combined with anthropogenic aerosols) contributes to 64-74% of total aerosols over the Himalayas. Dry deposition causes a substantial amount of dust aerosols (1-31 mg m(-2) day(-1)) to be deposited over the Himalayas, reducing the albedo by 0.3% on fresh snow and up to 2.7% on aged snow, causing a radiative forcing of 0.38-23.7 Wm(-2) at the top of the atmosphere. The Himalayan cryosphere may therefore experience large warming leading to snow melting and enhanced reduction in snow cover.
The perceptions and attitudes of community residents are a mirror of tourism development. Little research has been conducted on the effects of place attachment and emotional solidarity on community residents' attitudes toward tourism in China's glacier tourism-related areas. In this paper, we selected the southernmost marine glacier in China, Hailuogou Glacier Forest Park, as a case study, and constructed a structural equation model of residents' tourism perceptions and attitudes based on 358 valid questionnaires obtained from fieldwork. We analyzed the logical connection and influencing relationship between place attachment, residents' perceptions (residents' benefits and environmental perceptions), and community residents' attitudes (security, support, satisfaction), and explored countermeasures and suggestions for building a harmonious host-customer relationship in the Hailuogou area to improve glacier tourism. The results of the study show that the influence of place attachment and residents' perceptions on emotional solidarity is different from the degree of influence of emotional solidarity on residents' tourism attitudes, with the most significant positive influence of place attachment on emotional solidarity and the greatest influence of emotional solidarity on sense of security. Emotional solidarity had a certain mediating effect between place attachment, residents' perceptions, and residents' tourism attitudes. Significantly, emotional solidarity had the most fully mediated effect between place attachment and support, reaching 73.61%. The moderating effect of place attachment reflects that the higher the place attachment, the weaker the correlation between residents' perceptions and residents' tourism attitudes. Meanwhile, residents' tourism attitudes will weaken their influence with the increase in emotional solidarity. Based on the above results, relevant suggestions are made to provide a theoretical basis and decision-making reference for the development and management of glacier tourism destinations.
Aerosol direct radiative forcing is strongly dependent on aerosol distributions and aerosol types. A detailed understanding of such information is still missing at the Alpine region, which currently undergoes amplified climate warming. Our goal was to study the vertical variability of aerosol types within and above the Vipava valley (45.87 degrees N, 13.90 degrees E, 125 m a.s.1.) to reveal the vertical impact of each particular aerosol type on this region, a representative complex terrain in the Alpine region which often suffers from air pollution in the wintertime. This investigation was performed using the entire dataset of a dual-wavelength polarization Raman lidar system, which covers 33 nights from September to December 2017. The lidar provides measurements from midnight to early morning (typically from 00:00 to 06:00 CET) to provide aerosol-type dependent properties, which include particle linear depolarization ratio, lidar ratio at 355 nm and the aerosol backscatter Angstrom exponent between 355 nm and 1064 nm. These aerosol properties were compared with similar studies, and the aerosol types were identified by the measured aerosol optical properties. Primary anthropogenic aerosols within the valley are mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel, and traffic emissions. Natural aerosols, such as mineral dust and sea salt, are mostly transported over large distances. A mixture of two or more aerosol types was generally found. The aerosol characterization and statistical properties of vertical aerosol distributions were performed up to 3 km.
The Poland-AOD aerosol research network was established in 2011 to improve aerosol-climate interaction knowledge and provide a real-time and historical, comprehensive, and quantitative database for the aerosol optical properties distribution over Poland. The network consists of research institutions and private owners operating 10 measurement stations and an organization responsible for aerosol model transport simulations. Poland-AOD collaboration provides observations of spectral aerosol optical depth (AOD), angstrom ngstrom Exponent (AE), incoming shortwave (SW) and longwave (LW) radiation fluxes, vertical profiles of aerosol optical properties and surface aerosol scattering and absorption coefficient, as well as microphysical particle properties. Based on the radiative transfer model (RTM), the aerosol radiative forcing (ARF) and the heating rate are simulated. In addition, results from GEM-AQ and WRF-Chem models (e.g., aerosol mass mixing ratio and optical properties for several particle chemical components), and HYSPLIT back-trajectories are used to interpret the results of observation and to describe the 3D aerosol optical properties distribution. Results of Poland-AOD research indicate progressive improvement of air quality and at mospheric turbidity during the last decade. The AOD was reduced by about 0.02/10 yr (at 550 nm), which corresponds to positive trends in ARF. The estimated clear-sky ARF trend is 0.34 W/m(2)/10 yr and 0.68 W/m(2)/10 yr, respectively, at TOA and at Earth's surface. Therefore, reduction in aerosol load observed in Poland can significantly contribute to climate warming.
Atmospheric aerosols have been found to influence the development of planetary boundary layer (PBL) and hence to aggravate haze pollution in megacities. PBL height (PBLH) determines the vertical extent to which the most pollutant effectively disperses and is a key argument in pollution study. In this study, we quantitatively evaluate aerosol radiation effect on PBL, as well as assessment of surface cooling effect and atmosphere heating effect. All the data are measured at a site of Beijing from 2014 to 2017, of which PBLH is retrieved from micro pulse lidar and aerosol optical depth (AOD) from sunphotometer. Case study shows qualitatively that relative high aerosol load reduces PBLH, and in turn causes a high surface PM2.5 concentration. We preliminarily reveal the influential mechanism of aerosol on PBL. The influence of aerosol on the radiation flux of PBL is analyzed, with the correlation coefficient (R) of 0.938 between AOD and radiative forcing of BOA (RFBOA) and R = 0.43 between RFBOA and PBLH. Also, AOD is found to negatively correlate with PBLH (R = -0.41). With the increase of AOD, the cooling effect of surface is enhanced, and further impede the development of PBL. Due to aerosol-induced reduction of PBLH, near surface PM2.5 concentration surges and presents an exponential growth following AOD. Then, it is speculated and testified that the relationship between SSA (single scatting albedo) and PBLH would be determined by the location of absorbing aerosol within PBL. The upper PBL absorbing aerosol may decrease PBLH, while the lower absorbing aerosol appear to enhance PBLH. The study probably can provide effective observational evidence for understanding the effect of aerosol on PBL and be a reference of air pollution mitigation in Beijing and its surrounding areas. (C) 2019 Elsevier Ltd. All rights reserved.
Recent local-scale observations of glaciers, streams, and soil surfaces in the McMurdo Dry Valleys of Antarctica (MDV) have documented evidence for rapid ice loss, glacial thinning, and ground surface subsidence associated with melting of ground ice. To evaluate the extent, magnitude, and location of decadal-scale landscape change in the MDV, we collected airborne lidar elevation data in 2014-2015 and compared these data to a 2001-2002 airborne lidar campaign. This regional assessment of elevation change spans the recent acceleration of warming and melting observed by long-term meteorological and ecosystem response experiments, allowing us to assess the response of MDV surfaces to warming and potential thawing feedbacks. We find that locations of thermokarst subsidence are strongly associated with the presence of excess ground ice and with proximity to surface or shallow subsurface (active layer) water. Subsidence occurs across soil types and landforms, in low-lying, low-slope areas with impeded drainage and also high on steep valley walls. Glacier thinning is widespread and is associated with the growth of fine-scale roughness. Pond levels are rising in most closed-basin lakes in the MDV, across all microclimate zones. These observations highlight the continued importance of insolation-driven melting in the MDV. The regional melt pattern is consistent with an overall transition of water storage from the local cryosphere (glaciers, permafrost) to the hydrosphere (dosed basin lakes and ponds as well as the Ross Sea). We interpret this regional melting pattern to reflect a transition to Arctic and alpine-style, hydrologically mediated permafrost and glacial melt. (C) 2018 Published by Elsevier B.V.
Soil moisture has a pronounced effect on earth surface processes. Global soil moisture is strongly driven by climate, whereas at finer scales, the role of non-climatic drivers becomes more important. We provide insights into the significance of soil and land surface properties in landscape-scale soil moisture variation by utilizing high-resolution light detection and ranging (LiDAR) data and extensive field investigations. The data consist of 1200 study plots located in a high-latitude landscape of mountain tundra in north-western Finland. We measured the plots three times during growing season 2016 with a hand-held time-domain reflectometry sensor. To model soil moisture and its temporal variation, we used four statistical modelling methods: generalized linear models, generalized additive models, boosted regression trees, and random forests. The model fit of the soil moisture models were R-2 = 0.60 and root mean square error (RMSE) 8.04 VWC% on average, while the temporal variation models showed a lower fit of R-2 = 0.25 and RMSE 13.11 CV%. The predictive performances for the former were R-2 = 0.47 and RMSE 9.34 VWC%, and for the latter R-2 = 0.01 and RMSE 15.29 CV%. Results were similar across the modelling methods, demonstrating a consistent pattern. Soil moisture and its temporal variation showed strong heterogeneity over short distances; therefore, soil moisture modelling benefits from high-resolution predictors, such as LiDAR based variables. In the soil moisture models, the strongest predictor was SAGA (System for Automated Geoscientific Analyses) wetness index (SWI), based on a 1m(2) digital terrain model derived from LiDAR data, which outperformed soil predictors. Thus, our study supports the use of LiDAR based SWI in explaining fine-scale soil moisture variation. In the temporal variation models, the strongest predictor was the field-quantified organic layer depth variable. Our results show that spatial soil moisture predictions can be based on soil and land surface properties, yet the temporal models require further investigation. Copyright (c) 2017 John Wiley & Sons, Ltd.
This work presents a methodology for obtaining vertical profiles of aerosol single scattering properties based on a combination of different measurement techniques. The presented data were obtained under the iAREA (Impact of absorbing aerosols on radiative forcing in the European Arctic) campaigns conducted in Ny-angstrom lesund (Spitsbergen) during the spring seasons of 2015-2017. The retrieval uses in-situ observations of black carbon concentration and absorption coefficient measured by a micro-aethalometer AE-51 mounted onboard a tethered balloon, as well as remote sensing data obtained from sun photometer and lidar measurements. From a combination of the balloon-borne in-situ and the lidar data, we derived profiles of single scattering albedo (SSA) as well as absorption, extinction, and aerosol number concentration. Results have been obtained in an altitude range from about 400 m up to 1600 m a.s.l. and for cases with increased aerosol load during the Arctic haze seasons of 2015 and 2016. The main results consist of the observation of increasing values of equivalent black carbon (EBC) and absorption coefficient with altitude, and the opposite trend for aerosol concentration for particles larger than 0.3 mu m. SSA was retrieved with the use of lidar Raman and Klett algorithms for both 532 and 880 nm wavelengths. In most profiles, SSA shows relatively high temporal and altitude variability. Vertical variability of SSA computed from both methods is consistent; however, some discrepancy is related to Raman retrieval uncertainty and absorption coefficient estimation from AE-51. Typically, very low EBC concentration in Ny-angstrom lesund leads to large error in the absorbing coefficient. However, SSA uncertainty for both Raman and Klett algorithms seems to be reasonable, e.g. SSA of 0.98 and 0.95 relate to an error of +/- 0.01 and +/- 0.025, respectively. (C) 2017 Elsevier Ltd. All rights reserved.
A qualitative assessment on the effect of boundary layer dynamics in the estimation of clear sky black carbon (BC) radiative forcing has been made considering the debate on the lower bound and possible uncertainties in the aerosol radiative forcing estimation. Comprehensive measurements made on aerosol optical and physical properties, near surface BC mass concentrations and Lidar derived aerosol back scatter intensity profiles at three selected locations in India (Visakhapatnam, Kharagpur, and Kolkata) are utilized for this purpose. Sensitivity analysis carried out to estimate the errors in short wave (SW) BC forcing computation indicated that nonincorporation of diurnal changes in the boundary layer depth into the models may lead to over estimation of diurnally averaged (as the study is limited to short wave radiative forcing, diurnally averaged forcing refers to day-time averaged) BC forcing. The relative errors may vary between 7 to 70% depending on the season and the location changes in boundary layer depth day-time behaviour. The results reported in the present study, though specific to the study locations, clearly indicate that a more systematic approach is needed to investigate the sensitivity of aerosol radiative forcing to various atmospheric parameters and processes within the boundary layer, particularly at stations characterised by strong anthropogenic influence and large diurnal temperature variability that affect the boundary layer depth.