Atmospheric particulate matter (PM) as light-absorbing particles (LAPs) deposited to snow cover can result in early onset and rapid snow melting, challenging management of downstream water resources. We identified LAPs in 38 snow samples (water years 2013-2016) from the mountainous Upper Colorado River basin by comparing among laboratory-measured spectral reflectance, chemical, physical, and magnetic properties. Dust sample reflectance, averaged over the wavelength range of 0.35-2.50 mu m, varied by a factor of 1.9 (range, 0.2300-0.4444) and was suppressed mainly by three components: (a) carbonaceous matter measured as total organic carbon (1.6-22.5 wt. %) including inferred black carbon, natural organic matter, and carbon-based synthetic, black road-tire-wear particles, (b) dark rock and mineral particles, indicated by amounts of magnetite (0.11-0.37 wt. %) as their proxy, and (c) ferric oxide minerals identified by reflectance spectroscopy and magnetic properties. Fundamental compositional differences were associated with different iron oxide groups defined by dominant hematite, goethite, or magnetite. These differences in iron oxide mineralogy are attributed to temporally varying source-area contributions implying strong interannual changes in regional source behavior, dust-storm frequency, and (or) transport tracks. Observations of dust-storm activity in the western U.S. and particle-size averages for all samples (median, 25 mu m) indicated that regional dust from deserts dominated mineral-dust masses. Fugitive contaminants, nevertheless, contributed important amounts of LAPs from many types of anthropogenic sources.

Microplastics in drinking water captured widespread attention following reports of widespread detection around the world. Concerns have been raised about the potential adverse effects of microplastics in drinking water on human health. Given the widespread interest in this research topic, there is an urgent need to compile existing data and assess current knowledge. This paper provides a systematic review of studies on microplastics in drinking water, their evidence, key findings, knowledge gaps, and research needs. The data collected show that microplastics are widespread in drinking water, with large variations in reported concentrations. Standardized methodologies of sampling and analysis are urgently needed. There were more fibrous and fragmented microplastics, with the majority being <10 mu m in size and composed of polyester, polyethylene, polypropylene, and polystyrene. Little attention has been paid to the color of microplastics. More research is needed to understand the occurrence and transfer of microplastics throughout the water supply chain and the treatment efficiency of drinking water treatment plants (DWTPs). Methods capable of analyzing microplastics <10 mu m and nanoplastics are urgently needed. Potential ecological assessment models for microplastics currently in use need to be improved to take into account the complexity and specificity of microplastics.

Microplastic is an emerging contaminant of concern in soil globally due to its widespread and potential risks on the ecological system. Some basic issues such as the occurrence, source, and potential risks of microplastics in the soil are still open questions. These problems arise due to the lack of systematic and comprehensive analysis of microplastic in soils. Therefore, we comprehensively reviewed the current status of knowledge on microplastics in soil on detection, occurrence, characterization, source, and potential risk. Our review suggests that microplastics are ubiquitous in soil matrices globally. However, the research progress of microplastics in the soil is restricted by inherent technological inconsistencies and difficulties in analyzing particles in complex matrices, and studies on the occurrence and distribution of microplastics in soil environments remain very scarce, especially in Africa, South America, and Oceania. The consistency of the characteristics and composition of the microplastics in the aquatic environment and soil demonstrate they may share sources and exchange microplastics. Wide and varied sources of microplastic are constantly filling the soil, which causes the accumulation of microplastics in the soil. Studies on the effects and potential risks of microplastics in soil ecosystems are also reviewed. Limited research has shown that the combination and interaction of microplastics with contaminants they absorbed may affect soil health and function, and even migration along the food chain. The occurrence and impact of microplastic on the soil depend on the morphology, chemical components, and natural factors. We conclude that large research gaps exist in the quantification and estimation of regional emissions of microplastics in soil, factors affecting the concentration of microplastics, and microplastic disguising as soil carbon storage, which need more effort. (c) 2021 Elsevier B.V. All rights reserved.

Microplastic pollution has become an increasingly important environmental issue worldwide in recent years because of its ubiquitous presence in different environmental media and its potential to affect the health of organisms and ecosystems. Aquaculture contributes significantly to the world's food production and nutritional supply, especially in developing countries. Widespread occurrence of microplastics in aquaculture systems has raised great concern regarding aquaculture production and food safety issues of aquaculture products. China is a world leader in aquaculture production, with freshwater aquaculture accounting for 59.1% of total aquaculture production of the world in 2020. Therefore, this review mainly focuses on recent research progress related to microplastic pollution in freshwater aquaculture systems in China. Results from the literature show that microplastics are present in freshwater aquaculture systems at abundances comparable to natural waterbodies in China. Microplastics can be ingested and remain in the body of aquaculture products. Exposure to microplastics can adversely affect the health of aquatic organisms and aquatic ecosystem functions. However, risks of microplastics in real world environment remain uncertain. Consumption of freshwater aquaculture products is not a major pathway for human exposure to microplastics. To provide scientific guidance for governmental decision-making and pollution control, future work should focus on progress in toxicological methodology and understanding the impacts of microplastics at community and ecosystem levels.

There is a rising concern regarding the accumulation of microplastics in the aquatic ecosystems. However, compared to the marine environment, the occurrence, transport, and diffusion of microplastics in freshwater sediment are still open questions. This paper summarizes and compares the methods used in previous studies and provides suggestions for sampling and analysis of microplastics in freshwater sediment. This paper also reviews the findings on microplastics in freshwater sediment, including abundance, morphological characteristics, polymer types, sources, and factors affecting the abundance of microplastics in freshwater sediment. The results show that microplastics are ubiquitous in the investigated sediment of rivers, lakes, and reservoirs, with an abundance of 2-5 orders of magnitude across different regions. Low microplastics concentration was observed in the Ciwalengke River with an average abundance of 30.3 +/- 15.9 items/kg. In particular, an extremely high abundance of microplastics was recorded in the urban recipient in Norway reaching 12,000-200,000 items/kg. Fibers with particle size less than 1 mm are the dominant shape for microplastics in freshwater sediment. In addition, the most frequently recorded colors and types are white/transparent, and PE/PS, respectively. Finally, we conclude that the consistency of morphological characteristics and components of microplastics between the beach or marine sediments and freshwater sediments may be an indicator of these interlinkages and source-pathways. Microplastics in freshwater sediment need further research and exploration to identify its spatial and temporal variations and driving force through further field sampling and implementation of standard and uniform analytical methodologies. (C) 2020 Elsevier B.V. All rights reserved.

The cryosphere is the term used to describe the frozen areas of the Earth, including all forms of snow and ice, which are primarily influenced by anthropogenic pollutants through atmospheric transport. In this review, we described the current status of newly emergent pollutant-microplastics-in the snow and ice of typical cryospheric regions (e.g., Arctic, Antarctic, Alps, Tibetan Plateau, and Andes), discussed their transport pathways, and provided perspectives for future research. A brief summary of snow and ice sampling, pretreatment, and the identification of microplastics in cryospheric regions suggested that standard procedures were inadequate and urgently required improvement. Microplastics were widely distributed in snow and ice across the typical cryospheric regions, indicating the ubiquitous distribution of microplastics in such environments. However, the abundance, size distribution, shape, and polymer composition of the microplastics in snow and ice showed significant differences. Sea ice was especially important for the temporal storage, transport, and release of microplastics in the Arctic and Antarctic. Microplastics in land snow cover and mountain glaciers emphasized the importance of atmospheric transport in the transferal of microplastics to cryospheric regions. In particular, the non-polar cryospheric regions (e.g., Tibetan Plateau, Andes, or Alps) were highlighted as important receptors of mid-latitude emissions of microplastics, which might indicate a future climatic risk considering the ability of microplastics to absorb radiation and accelerate the melting of snow. Microplastics retrieved from mountain glacier ice cores may also provide new insights into the historical variations of anthropogenic pollutants. The potential impact of microplastics in snow and ice on the carbon cycle and the climatic risk needs to be further addressed in the future.

Microplastics have recently been detected in the atmosphere of urban, suburban, and even remote areas far away from source regions of microplastics, suggesting the potential long-distance atmospheric transport for microplastics. There still exist questions regarding the occurrence, fate, transport, and effect of atmospheric microplastics. These questions arise due to limited physical analysis and understanding of atmospheric microplastic pollution in conjunction with a lack of standardized sampling and identification methods. This paper reviews the current status of knowledge on atmospheric microplastics, the methods for sample collection, analysis and detection. We review and compare the methods used in the previous studies and provide recommendations for atmospheric microplastic sampling and measurement. Furthermore, we summarize the findings related to atmospheric microplastic characteristics, including abundance, size, shapes, colours, and polymer types. Microplastics occur in the atmosphere from urban to remote areas, with an abundance/deposition spanning 1-3 orders of magnitude across different sites. Fibres and fragments are the most frequently reported shapes and the types of plastic which generally aligns with world plastic demand. We conclude that atmospheric microplastics require further research and greater understanding to identify its global distributions and potential exposure to human health through further field sampling and implementation of standardized analytical protocols.

Microplastics are widely detected in terrestrial environments. However, microplastic features in the soil of remote areas are still sparse. In this study, microplastic pollution in soil across the Tibetan Plateau was systematically investigated. The results revealed that microplastic was ubiquitous in the soil of the Tibetan Plateau with an average abundance of 47.12 items/kg-dry weight (range: 5-340 items/kg). Compared with the published data of soil microplastic pollution in other regions, the microplastic pollution in the Tibetan Plateau was relatively low. Fibers represented 43.54% of microplastic particles detected, followed by fragments (32.20%) and films (23.78%). They mainly consisted of polyvinyl chloride, polyethylene, polypropylene, and polystyrene. Transparent and white microplastics were prevalent, and small microplastics (50-500 mu m) occupied approximately 66% of all microplastics. High values of microplastics were found near Lhasa, Naqu, and Linzhi. Furthermore, microplastic pollution was found to be negatively related to the distance to the nearest city (p < 0.01), wind velocity (p = 0.014), altitude (p = 0.181), yet positively related to precipitation (p = 0.024). This work presents new insights into the magnitude of microplastics contamination in the soil across the Tibetan Plateau and supplies valuable data for future research on ecotoxicology, ecosystem impacts, and earth system feedback of microplastics on terrestrial ecosystems.

Microplastics (MPs) pollution has become a serious environmental issue of growing global concern due to the increasing plastic production and usage. Under climate warming, the cryosphere, defined as the part of Earth's layer characterized by the low temperatures and the presence of frozen water, has been expe-riencing significant changes. The Arctic cryosphere (e.g., sea ice, snow cover, Greenland ice sheet, per-mafrost) can store and release pollutants into environments, making Arctic an important temporal sink and source of MPs. Here, we summarized the distributions of MPs in Arctic snow, sea ice, seawater, rivers, and sediments, to illustrate their potential sources, transport pathways, storage and release, and possible effects in this sentinel region. Items concentrations of MPs in snow and ice varied about 1-6 orders of magnitude in different regions, which were mostly attributed to the different sampling and measurement methods, and potential sources of MPs. MPs concentrations from Arctic seawater, river/ lake water, and sediments also fluctuated largely, ranging from several items of per unit to >40,000 items m-3, 100 items m-3, and 10,000 items kg -1 dw, respectively. Arctic land snow cover can be a temporal storage of MPs, with MPs deposition flux of about (4.9-14.26) x 108 items km -2 yr-1. MPs transported by rivers to Arctic ocean was estimated to be approximately 8-48 ton/yr, with discharge flux of MPs at about (1.65-9.35) x 108 items/s. Average storage of MPs in sea ice was estimated to be about 6.1x1018 items, with annual release of about 5.1x1018 items. Atmospheric transport of MPs from long-distance terrestrial sources contributed significantly to MPs deposition in Arctic land snow cover, sea ice and oceanic surface waters. Arctic Great Rivers can flow MPs into the Arctic Ocean. Sea ice can temporally store, transport and then release MPs in the surrounded environment. Ocean currents from the Atlantic brought high concentrations of MPs into the Arctic. However, there existed large uncertain-ties of estimation on the storage and release of MPs in Arctic cryosphere owing to the hypothesis of aver-age MPs concentrations. Meanwhile, representatives of MPs data across the large Arctic region should be mutually verified with in situ observations and modeling. Therefore, we suggested that systematic mon-itoring MPs in the Arctic cryosphere, potential threats on Arctic ecosystems, and the carbon cycle under increasing Arctic warming, are urgently needed to be studied in future.(c) 2023 China University of Geosciences (Beijing) and Peking University. Production and hosting by Elsevier B.V. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/ licenses/by-nc-nd/4.0/).