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The significant uncertainties of Black Carbon (BC) radiative forcing are becoming an obstacle to the evaluation of their impacts and mitigation measures. One of the crucial reasons for this uncertainty could be the poorly constrained BC vertical profile. The BC has a lifetime of a few days to weeks and there is a clear pointer that it can be vertically transported through convection besides the horizontal advection. The present study aims for the intercomparison between the BC mass concentrations obtained through the aircraft-based observations and that derived from the selected Copernicus Atmosphere Monitoring Service (CAMS) reanalysis data over the three different locations of India, which is one of the largest emitters of BC aerosols. The aircraft-based BC observations were conducted from 0.5 to 7 km altitudes using Aethalometer during CAIPEEX (Cloud Aerosol Interaction and Precipitation Enhancement Experiment) Phase I campaigns from June to September 2009. The output of the present study suggests the CAMS reanalysis data significantly underestimated BC mass throughout the vertical profile with an average mass normalized mean bias of greater than -70% at all three locations. Furthermore, the vertical radiative forcing and heating rates of BC were also calculated for both observation and reanalysis data. The output depicts the net forcing due to CAMS simulated BC in all the layers were 1-12 folds lower over all the study regions compared with observed BC aerosols. Likewise, the estimated mean biases in heating rate were in the range of -0.001 to -0.190 K day(-1) for all the vertical layers over the study locations. The possible reasons for these disparities could be poorly constrained emissions, especially aircraft emissions and/or their transformation schemes in aerosol modules. The present study emphasized that the validation of the vertical profile is also an essential factor for better constraints of the BC aerosols in climate models.

期刊论文 2024-12-01 DOI: 10.1016/j.jastp.2024.106358 ISSN: 1364-6826

Aerosol single-scattering albedo (SSA) is the most critical factor for the accurately calculating of aerosol radiative effects, however, the observation of vertical profiles of SSA is difficult to realize. Current assessments of aerosol radiative effects remain uncertain because of the lack of long-term, high-resolution vertical profiles of SSA observations. High-resolution SSA vertical profiles were observed in a semi-arid region of Northwest China during winter using a tethered balloon. The observed SSA vertical profiles were used to calculate the aerosol direct radiative forcing and radiative heating rates. Significant differences in the calculated radiative forcing were found (e.g., a 48.3% relative difference for the heating effect in the atmosphere at 14:00) between the observed SSA profiles and the constant assumption with SSA = 0.90. Diurnal variations in the vertical distribution of SSA decisively influenced direct radiative forcing of aerosols. Furthermore, high-resolution vertical profiles of absorbing aerosols and meteorological parameters provide robust observational evidence of the heating effect of an elevated absorbing aerosol layer. This study provides a more accurate calculation of aerosol radiative forcing using observed aerosol SSA profiles. The scarcity of single-scattering albedo (SSA) observations is the most critical factor limiting the accurate calculations of aerosol radiative effects. A tethered balloon platform was used to obtain long-term, high-resolution observations of the SSA and estimate aerosols' radiative effects. The relative differences in the heating rate and direct radiative forcing calculations using the observed SSA and a constant assumed SSA (i.e., ignoring the vertical distribution of absorbing aerosols) were quantified. The effects of diurnal variations in the vertical distribution of SSA on aerosol direct radiative forcing are summarized. This study has important scientific implications for assessing the radiative effects of aerosols in semi-arid regions, that are highly sensitive to climate change. Tethered balloon observations acquired high-resolution vertical aerosol single-scattering albedo (SSA) profiles The assumed SSA profiles caused a 48.3% relative error in radiative forcing in the atmosphere compared to the observed profiles at 14:00 A robust observational evidence of atmospheric heating by absorbing aerosols above the boundary layer was provided

期刊论文 2024-07-28 DOI: 10.1029/2023JD040605 ISSN: 2169-897X

Vertical electrical sounding method is an express and most accurate method for measuring and analysing the resistivity through the soil profile. As a result of climate change, permafrost is melting, which leads to a significant transformation of landscapes, both natural and anthropogenically transformed. In the vulnerable environments of the Arctic region (long recovery after anthropogenic impact), this method allows to determine the active layer thickness and the heterogeneity in the soil structure without disturbing of the soil cover. This method is based on the measurement of electrical resistivity in the soil, the data obtained were processed in the form of one dimensional model. In the course of field research, the heterogeneous islands of the Lena River Delta were investigated. Complex soil investigations using the method of vertical electrical sensing allows to fully assess the most important properties of cryogenic soils formed in the delta complex of the Lena River. As a result of the work, the modeled boundaries of the active layer were determined, which were confirmed during the laying of soil transects, as well as the main physical and chemical parameters of soils. During the vertical electrical sounding observation an inhomogeneity in the distribution of resistivity under a drained lake was found, which may correspond to the presence of a talik or a layer of salt unfrozen water in a permafrost. Due to the change in the soil horizons, there is a sharp change in the electrical resistivity indicator occur, which corresponds to the change from soil to frozen rock. The paper contains 6 Figures, 3 Tables and 37 References.

期刊论文 2023-09-01 DOI: 10.17223/19988591/63/2 ISSN: 1998-8591

With Tibetan Plateau higher than 4 km to the west, the location of Sichuan Basin is unique all around the world and provides a good platform to study air pollution in the urban agglomerations over the complex terrain. To fill in the blanks on vertical distributions of PM1 (the particles smaller than 1 mu m) and carbonaceous aerosols within the basin, by means of high topographic relief, PM1 were off-line sampled during 20 January to 2 February 2018 at eight sites with increasing altitudes from the basin to southeastern margins of the Tibetan Plateau. The regional potential sources for each site were revealed by Hybrid-Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model and concentration-weighted trajectory (CWT) method. The lowest carbonaceous aerosol levels occurred at Lixian, while the highest OC (organic carbon) (EC, elemental carbon) was at Hongyuan (the altitude of 3500 m) (Ande, a rural site) due to more primary emissions. The pollutants inside the basin can be transported the altitudes from 2 km to 3 km by vertical dispersion, but they cannot be dispersed to higher altitudes. The vertical stratification of the pollutants was obvious and easily formed high-low-high pattern from Sichuan Basin to southeastern Tibetan Plateau, especially during highly polluted episodes. The regional potential sources significantly varied as the increased altitudes. Regional pollution was significant inside the basin. The sources at the altitudes from 2 km to 3 km originated from southeastern margins of the Plateau and surrounding cities, while those at higher altitudes were transported from southeastern margins of the Plateau. The impact of basic meteorological variables (temperature, wind speed and vapor pressure) on carbonaceous aerosols was opposite between the basin and Plateau sites. This study was essential to understanding formation mechanisms of severe pollution episodes and thus to making control measures for the urban agglomerations inside the mountainous terrain.

期刊论文 2023-08-15 DOI: http://dx.doi.org/10.1016/j.atmosenv.2020.117269 ISSN: 1352-2310

Atmospheric aerosols have important impacts on global radiative forcing, air pollution, and human health. This study investigated the optical and physical properties of aerosol layers over Australia from 2007 to 2019 using the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) Level 2 aerosol products. Australia was divided into three sub-regions (western highlands, central plains, and eastern ranges). Interannual and seasonal optical property variations in aerosol layers in the three sub-regions were analyzed and compared. Results showed that annual mean values of AOD(L) (lowest aerosol layer AOD) and AOD(T) (total AOD of all aerosol layers) were always higher in the eastern ranges region than the other two regions from 2007 to 2019. The reason could be that Australian population was predominantly located in the eastern ranges region, where more human activities could bring significant aerosol loadings. B-L (base height of the lowest aerosol layer), H-L (top height of the lowest aerosol layer), and H-H (top height of the highest aerosol layer) all showed trends of western highlands > eastern mountains > central plains, indicating that the higher the elevation, the higher the B-L, H-L, and H-H. T-L (thickness of the lowest aerosol layer) was higher during the day than at night, which might account for increased diurnal atmospheric convection and nocturnal aerosol deposition. DRL (depolarization ratio of the lowest aerosol layer) was higher in the western highlands and central plains than the eastern mountains, probably because these two regions have large deserts with more irregularly shaped dust aerosols. CRL (color ratio of the lowest aerosol layer) had slightly higher values in the eastern ranges than the other two regions, probably due to the wet climate of the eastern ranges, where aerosols were more hygroscopic and had larger particle sizes. This study can provide technical support for the control and management of regional air pollutants.

期刊论文 2023-07-01 DOI: 10.3390/atmos14071145

Limited by the scarcity of in situ vertical observation data, the influences of biomass burning in Southeast Asia on major atmospheric carbonaceous compositions in downwind regions have not been thoroughly studied. In this study, aircraft observations were performed to obtain high time-resolved in situ vertical distributions of black carbon (BC) as well as carbon monoxide (CO) and carbon dioxide (CO2). Four types of profiles were revealed: Mode I (from 2000 to 3000 m, the BC, CO and CO2 concentrations were enhanced), Mode II (with increasing altitude, the BC, CO and CO2 concentrations almost decreased), Mode III (inhomogeneous vertical BC, CO and CO2 profiles with BC peaks were observed from 2500 to 3000 m) and Mode IV (the BC, CO and CO2 concentrations increased above 1500 m). Furthermore, simulations were conducted to calculate radiative forcing (RF) caused by BC and study the heating rate (HR) of BC in combination with the vertical BC profiles. A larger BC distribution in the atmosphere re-sulted in a sharp RF change from negative to positive values, imposing a nonnegligible influence on the atmospheric temperature profile, with maximum HR values ranging from 0.4 to 5.8 K/day. The values of the absorption Angstrom exponent (AAE) were 1.46 +/- 0.11 and 1.48 +/- 0.17 at altitudes from 1000 to 2000 and 2000-3000 m, respectively. The average BC light absorption coefficient at the 370 nm wavelength (alpha BC (370)) accounted for 50.3 %-76.8 % of the alpha (370), while the brown carbon (BrC) light absorption coefficient at the 370 nm wavelength (alpha BrC (370)) contrib-uted 23.2 %-49.7 % to the alpha (370) at altitudes of 1000-2000 m. At altitudes of 2000-3000 m, alpha BC (370) and alpha BrC (370) contributed 43.8 %-88.2 % and 11.8 %-56.2 % to the alpha (370), respectively. These findings show that calculations that consider the surface BC concentration but ignore the vertical BC distribution could result in massive uncertainties in estimating the RF and HR caused by BC. This study helped achieve a deeper understanding of the influences of biomass burning over the region of Southeast Asia on the profiles of atmospheric carbonaceous compositions and atmospheric BC absorption and its warming effect.

期刊论文 2023-01-20 DOI: 10.1016/j.scitotenv.2022.159232 ISSN: 0048-9697

Owing to global warming, the rise in sea temperature is causing degradation of submarine permafrost, which has an impact on the seismic responses of submarine strata. Based on the revised dynamics of nearly saturated frozen porous media, a simplified model of the vertical seismic responses of submarine permafrost is established considering the degradation of its upper layer, and an analytical solution is obtained using the Laplace transform method. The governing equation of a single-degree-of-freedom system on the seafloor is further proposed, and the vertical response spectrum is obtained using the numerical inverse transformation method. The numerical results show that the vertical ground motions of the seafloor agree well with those of saturated and nearly saturated soil layers with a free surface on land and under deep-water conditions. Parametric studies show that saturation strongly affects the vertical ground motions of the seafloor, and this effect is closely related to the water depth ratio. In addition, the structural stratum parameters, including the active layer thickness ratio, permafrost thickness, and temperature, have significant effects on the vertical ground motions of the seafloor and the vertical response spectrum of the submarine lumped parameter system. Therefore, attention should be paid to the impact of submarine permafrost degradation on the vertical seismic responses of oil and gas exploitation systems in polar oceans. (c) 2022 Elsevier Ltd. All rights reserved.

期刊论文 2022-12-01 DOI: 10.1016/j.gete.2022.100402 ISSN: 2352-3808

Aerosol direct radiative forcing is strongly dependent on aerosol distributions and aerosol types. A detailed understanding of such information is still missing at the Alpine region, which currently undergoes amplified climate warming. Our goal was to study the vertical variability of aerosol types within and above the Vipava valley (45.87 degrees N, 13.90 degrees E, 125 m a.s.1.) to reveal the vertical impact of each particular aerosol type on this region, a representative complex terrain in the Alpine region which often suffers from air pollution in the wintertime. This investigation was performed using the entire dataset of a dual-wavelength polarization Raman lidar system, which covers 33 nights from September to December 2017. The lidar provides measurements from midnight to early morning (typically from 00:00 to 06:00 CET) to provide aerosol-type dependent properties, which include particle linear depolarization ratio, lidar ratio at 355 nm and the aerosol backscatter Angstrom exponent between 355 nm and 1064 nm. These aerosol properties were compared with similar studies, and the aerosol types were identified by the measured aerosol optical properties. Primary anthropogenic aerosols within the valley are mainly emitted from two sources: individual domestic heating systems, which mostly use biomass fuel, and traffic emissions. Natural aerosols, such as mineral dust and sea salt, are mostly transported over large distances. A mixture of two or more aerosol types was generally found. The aerosol characterization and statistical properties of vertical aerosol distributions were performed up to 3 km.

期刊论文 2022-07-01 DOI: 10.3390/rs14143482

Soil microorganisms are crucial contributors to the function of permafrost ecosystems, as well as the regulation of biogeochemical cycles. However, little is known about the distribution patterns and drivers of high-latitude permafrost microbial communities subject to climate change and human activities. In this study, the vertical distribution patterns of soil bacterial communities in the Greater Khingan Mountain permafrost region were systematically analyzed via Illumina Miseq high-throughput sequencing. Bacterial diversity in the active layer was significantly higher than in the permafrost layer. Principal coordinate analysis (PCoA) indicated that the bacterial community structure in the active layer and the permafrost layer was completely separated. Permutational multivariate analysis of variance (PERMANOVA) detected statistically significant differentiation across the different depths. The relative abundance of the dominant phyla Chloroflexi (17.92%-52.79%) and Actinobacteria (6.34%-34.52%) was significantly higher in the permafrost layer than in the active layer, whereas that of Acidobacteria (4.98%-38.82%) exhibited the opposite trend, and the abundance of Proteobacteria (2.49%-22.51%) generally decreased with depth. More importantly, the abundance of bacteria linked to human infectious diseases was significantly higher in the permafrost layer according to Tax4Fun prediction analysis. Redundancy analysis (RDA) showed that ammonium nitrogen (NH4+-N), total organic carbon (TOC), and total phosphorus (TP) were major factors affecting the bacterial community composition. Collectively, our findings provide insights into the soil bacterial vertical distribution patterns and major environmental drivers in high-latitude permafrost regions, which is key to grasping the response of cold region ecosystem processes to global climate changes.

期刊论文 2022-07-01 DOI: 10.1002/ece3.9106 ISSN: 2045-7758

Due to the extreme, harsh natural environment in the Himalayas higher than 8000 m above sea level (asl) long-term and continuous meteorological observation is still a great challenge, and little is known about water vapor transport in this extremely high region. Based on the Automatic Weather Stations (AWSs) at 3810 m, 5315 m, 6464 m, 7945 m and 8430 m asl on the southern slope of Mt. Everest, this study investigates the meteorological characteristics and water vapor transport in the Mt. Everest region from June 2019 to June 2021. The results show that (1) with the increase of altitude, the temperature lapse rate becomes deeper from -4.7 degrees C km(-1) to -8.1 degrees C km(-1); (2) the relative humidity increases significantly in summer, and precipitation during the monsoon period accounts for more than 70% of the annual total; and (3) during the monsoon in 2020, the number of days with negative daily water vapor divergence in the whole layer accounted for 31% at the height from ground to 350 hPa, and the moisture amount transported through water vapor convergence was about 122 mm. The study indicates that, with sufficient moisture supply, strong water vapor convergence and a relatively large vertical velocity, a small amount of water vapor can climb to an extreme height and be transported from the southern to the northern slope of the Himalayas.

期刊论文 2022-06-01 DOI: http://dx.doi.org/10.3390/w14111671
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